同轴气化通道煤炭地下气化产品气热值分析及预测

Analysis and prediction of gas calorific value of coal underground gasification products from coaxial gasification channel

  • 摘要: 在煤炭地下气化(UCG)过程中,操作参数和煤的性质不同会导致UCG系统表现出不同的气化过程,产品气热值稳定产出一定时间后也会出现下降趋势。在人工煤层构建2种同轴煤炭地下气化模型,研究同轴气化通道对生成气化产物中气体成分及热值的影响,并对比分析压力、气化剂流量、气体组分对热值的影响,提出Informer热值预测模型,使用ERMSEMAR2作为评价指标,将结果与4种机器学习模型(LSTM、MLP、RNN和ARIMA)进行比较,对比分析不同预测时间长度下产品气热值的实际值、预测值及误差。结果表明:不同的同轴气化通道能够影响气化效果,改变气化通道延展长度,可以改变产出气体中可燃气体组分比例。同轴模型1产品气中有效气体组分(CO、H2和CH4)的体积分数为33.45%,平均热值为 4.68 MJ/Nm3;同轴模型2产品气中有效气体组分的体积分数为35.09%,平均热值为 4.75 MJ/Nm3。相比同轴模型 1 ,在同轴模型 2 中,H2的体积分数由6.17%提高至8.10%,而CH4的体积分数则由1.19%减少至0.61%。调整气化剂流量会改变气化炉的平衡状态,从而短暂提高产品气热值。与其他参考模型相比,EMA下降了22.42%~42.78%,ERMS下降了15.38%~30.49%,Informer热值预测模型表现优异,预测精度高。模型在不同的数据集、预测长度和采样频率下均具有较高的预测精度。同轴模型1数据集的平均误差为8%~18%,同轴模型 2 数据集的平均误差为5%~12%。Informer模型在预测不同时间段热值曲线时,能够有效预测出热值变化的不同趋势,且可以预测参数调整后的系统表现。

     

    Abstract: In the underground coal gasification (UCG) process, different operating parameters and coal properties can cause the UCG system to exhibit different gasification processes, and the calorific value of the product gas will also show a decreasing trend after a certain time of stable output. Two coaxial coal underground gasification models are constructed in an artificial coal seam to study the effects of coaxial gasification channels on the gas composition and calorific value of the generated gasification products, and the effects of pressure, gasifier flow rate, and gas components on the calorific value are comparatively analyzed. The Informer calorific value prediction model is proposed, using ERMS, EMA and R2 as evaluation indexes, and the results are compared with four machine learning models (LSTM, MLP, RNN, and ARIMA) to comparatively analyze the actual and predicted values and errors of the calorific value of the product gas under different prediction time lengths. The results show that different coaxial gasification channels can affect the gasification effect, and changing the extended length of gasification channels can change the proportion of combustible gas components in the product gas. In coaxial model 1, the volume fraction of effective gas components (CO, H2 and CH4) in the product gas was 33.45%, and the average calorific value was 4.68 MJ/Nm3; in coaxial model 2, the volume fraction of effective gas components in the product gas was 35.09%, and the average calorific value was 4.75 MJ/Nm3. Compared with the coaxial model 1, the volume fraction of H2 in the coaxial model 2 increased from 6.17% to 8.10%, while the volume fraction of CH4 decreases from 1.19% to 0.61%. Adjusting the gasifier flow rate changes the gasifier equilibrium, which transiently increases changes the calorific value of the product gas. Compared with other reference models, the EMA decreased by 22.42%-42.78%, and the ERMS decreased by 15.38%-30.49%. The Informer calorific value prediction model performed outstandingly with high prediction accuracy. The model has high prediction accuracy across different datasets, prediction lengths, and sampling frequencies. The average error for the coaxial model 1 dataset is in the range of 8%-18%, and the average error for the coaxial model 2 dataset is in the range of 5%-12%. The Informer model is able to effectively predict the different trends of thermal value changes when predicting thermal value curves in different time periods, and it can also predict the performance of the system after parameter adjustment.

     

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